Wrinkled 3D MoS2/RGO/NC composite microspheres: Optimal composition and microwave absorbing properties

Zihao Liu; Yihao Fan; Zhigang Liu; Qiuyu Zhang; Baoliang Zhang

doi:10.1016/j.compositesa.2022.107119

Wrinkled 3D MoS₂/RGO/NC composite microspheres: Optimal composition and microwave absorbing properties

Zihao Liu, Yihao Fan, Zhigang Liu, Qiuyu Zhang, Baoliang Zhang

School of Chemistry and Chemical Engineering

Research output: Contribution to journal › Article › peer-review

37 Scopus citations

Abstract

MoS₂ and graphene oxide (GO) are assembled into three-dimensional MoS₂/GO wrinkled microspheres by one-step ultrasonic spray technique. MoS₂/RGO/NC wrinkled microspheres are obtained after carbonization of MoS₂/GO coated with polydopamine (PDA) shell. The microspheres exhibited excellent microwave absorbing properties benefiting from its complex structure, complementary loss mechanisms and great impedance matching. The minimum reflection loss (RL_min) of MoS₂/RGO/NC wrinkled microspheres can obtain −60.4 dB@8.4 GHz, and the corresponding thickness is 3.1 mm. The optimal MoS₂ to GO feed ratio is 1:2. Adjusting the composition of the microspheres, the material effective absorption bandwidth (EAB) is up to 6.1 GHz (11.9–18.0 GHz) at a thickness of 2.9 mm. The optimized assembly of the three materials led to the further enhancement of the microsphere performance owe to the special morphology design as well as the splendid electrical conductivity. This work offers an efficacious reference idea for the device of novel and significant wave absorbers.

Original language	English
Article number	107119
Journal	Composites Part A: Applied Science and Manufacturing
Volume	161
DOIs	https://doi.org/10.1016/j.compositesa.2022.107119
State	Published - Oct 2022

Keywords

A. Nanocomposites
B. Microstructures
E. Assembly
MoS nanosheet

Access to Document

10.1016/j.compositesa.2022.107119

Cite this

@article{5ccdaf43a185442193f54adb5e8de06f,

title = "Wrinkled 3D MoS2/RGO/NC composite microspheres: Optimal composition and microwave absorbing properties",

abstract = "MoS2 and graphene oxide (GO) are assembled into three-dimensional MoS2/GO wrinkled microspheres by one-step ultrasonic spray technique. MoS2/RGO/NC wrinkled microspheres are obtained after carbonization of MoS2/GO coated with polydopamine (PDA) shell. The microspheres exhibited excellent microwave absorbing properties benefiting from its complex structure, complementary loss mechanisms and great impedance matching. The minimum reflection loss (RLmin) of MoS2/RGO/NC wrinkled microspheres can obtain −60.4 dB@8.4 GHz, and the corresponding thickness is 3.1 mm. The optimal MoS2 to GO feed ratio is 1:2. Adjusting the composition of the microspheres, the material effective absorption bandwidth (EAB) is up to 6.1 GHz (11.9–18.0 GHz) at a thickness of 2.9 mm. The optimized assembly of the three materials led to the further enhancement of the microsphere performance owe to the special morphology design as well as the splendid electrical conductivity. This work offers an efficacious reference idea for the device of novel and significant wave absorbers.",

keywords = "A. Nanocomposites, B. Microstructures, E. Assembly, MoS nanosheet",

author = "Zihao Liu and Yihao Fan and Zhigang Liu and Qiuyu Zhang and Baoliang Zhang",

note = "Publisher Copyright: {\textcopyright} 2022 Elsevier Ltd",

year = "2022",

month = oct,

doi = "10.1016/j.compositesa.2022.107119",

language = "英语",

volume = "161",

journal = "Composites Part A: Applied Science and Manufacturing",

issn = "1359-835X",

publisher = "Elsevier Ltd",

}

TY - JOUR

T1 - Wrinkled 3D MoS2/RGO/NC composite microspheres

T2 - Optimal composition and microwave absorbing properties

AU - Liu, Zihao

AU - Fan, Yihao

AU - Liu, Zhigang

AU - Zhang, Qiuyu

AU - Zhang, Baoliang

PY - 2022/10

Y1 - 2022/10

N2 - MoS2 and graphene oxide (GO) are assembled into three-dimensional MoS2/GO wrinkled microspheres by one-step ultrasonic spray technique. MoS2/RGO/NC wrinkled microspheres are obtained after carbonization of MoS2/GO coated with polydopamine (PDA) shell. The microspheres exhibited excellent microwave absorbing properties benefiting from its complex structure, complementary loss mechanisms and great impedance matching. The minimum reflection loss (RLmin) of MoS2/RGO/NC wrinkled microspheres can obtain −60.4 dB@8.4 GHz, and the corresponding thickness is 3.1 mm. The optimal MoS2 to GO feed ratio is 1:2. Adjusting the composition of the microspheres, the material effective absorption bandwidth (EAB) is up to 6.1 GHz (11.9–18.0 GHz) at a thickness of 2.9 mm. The optimized assembly of the three materials led to the further enhancement of the microsphere performance owe to the special morphology design as well as the splendid electrical conductivity. This work offers an efficacious reference idea for the device of novel and significant wave absorbers.

AB - MoS2 and graphene oxide (GO) are assembled into three-dimensional MoS2/GO wrinkled microspheres by one-step ultrasonic spray technique. MoS2/RGO/NC wrinkled microspheres are obtained after carbonization of MoS2/GO coated with polydopamine (PDA) shell. The microspheres exhibited excellent microwave absorbing properties benefiting from its complex structure, complementary loss mechanisms and great impedance matching. The minimum reflection loss (RLmin) of MoS2/RGO/NC wrinkled microspheres can obtain −60.4 dB@8.4 GHz, and the corresponding thickness is 3.1 mm. The optimal MoS2 to GO feed ratio is 1:2. Adjusting the composition of the microspheres, the material effective absorption bandwidth (EAB) is up to 6.1 GHz (11.9–18.0 GHz) at a thickness of 2.9 mm. The optimized assembly of the three materials led to the further enhancement of the microsphere performance owe to the special morphology design as well as the splendid electrical conductivity. This work offers an efficacious reference idea for the device of novel and significant wave absorbers.

KW - A. Nanocomposites

KW - B. Microstructures

KW - E. Assembly

KW - MoS nanosheet

UR - http://www.scopus.com/inward/record.url?scp=85135370623&partnerID=8YFLogxK

U2 - 10.1016/j.compositesa.2022.107119

DO - 10.1016/j.compositesa.2022.107119

M3 - 文章

AN - SCOPUS:85135370623

SN - 1359-835X

VL - 161

JO - Composites Part A: Applied Science and Manufacturing

JF - Composites Part A: Applied Science and Manufacturing

M1 - 107119

ER -

Wrinkled 3D MoS₂/RGO/NC composite microspheres: Optimal composition and microwave absorbing properties

Abstract

Keywords

Access to Document

Other files and links

Fingerprint

Cite this