Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities

Ruoyu Zhao; Teng Wang; Junjun Li; Yongxia Shi; Man Hou; Yong Yang; Zhicheng Zhang; Shengbin Lei

doi:10.1007/s12274-022-5307-1

Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities

Ruoyu Zhao, Teng Wang, Junjun Li, Yongxia Shi, Man Hou, Yong Yang, Zhicheng Zhang, Shengbin Lei

School of Chemistry and Chemical Engineering

Research output: Contribution to journal › Review article › peer-review

25 Scopus citations

Abstract

Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of the catalytic sites in two-dimensional (2D) COF-based electrocatalysts and analyzes the relationship between 2D COF structure and their electrocatalytic performances. In particular, the recent progress in the field of 2D COFs as electrocatalysts is comprehensively summarized. Finally, we discuss the current shortcomings and challenges on tailoring 2D COF for high-performance electrocatalysts in details, and look forward to promoting more researches on 2D COF-based electrocatalysts.[Figure not available: see fulltext.].

Original language	English
Pages (from-to)	8570-8595
Number of pages	26
Journal	Nano Research
Volume	16
Issue number	7
DOIs	https://doi.org/10.1007/s12274-022-5307-1
State	Published - Jul 2023

Keywords

active centers
covalent organic frameworks
electrocatalysts
two-dimensional

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10.1007/s12274-022-5307-1

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title = "Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities",

abstract = "Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of the catalytic sites in two-dimensional (2D) COF-based electrocatalysts and analyzes the relationship between 2D COF structure and their electrocatalytic performances. In particular, the recent progress in the field of 2D COFs as electrocatalysts is comprehensively summarized. Finally, we discuss the current shortcomings and challenges on tailoring 2D COF for high-performance electrocatalysts in details, and look forward to promoting more researches on 2D COF-based electrocatalysts.[Figure not available: see fulltext.].",

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author = "Ruoyu Zhao and Teng Wang and Junjun Li and Yongxia Shi and Man Hou and Yong Yang and Zhicheng Zhang and Shengbin Lei",

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T1 - Two-dimensional covalent organic frameworks for electrocatalysis

T2 - Achievements, challenges, and opportunities

AU - Zhao, Ruoyu

AU - Wang, Teng

AU - Li, Junjun

AU - Shi, Yongxia

AU - Hou, Man

AU - Yang, Yong

AU - Zhang, Zhicheng

AU - Lei, Shengbin

PY - 2023/7

Y1 - 2023/7

N2 - Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of the catalytic sites in two-dimensional (2D) COF-based electrocatalysts and analyzes the relationship between 2D COF structure and their electrocatalytic performances. In particular, the recent progress in the field of 2D COFs as electrocatalysts is comprehensively summarized. Finally, we discuss the current shortcomings and challenges on tailoring 2D COF for high-performance electrocatalysts in details, and look forward to promoting more researches on 2D COF-based electrocatalysts.[Figure not available: see fulltext.].

AB - Covalent organic frameworks (COFs) represent an emerging class of crystalline porous polymers with high porosity, good stability, and adjustable structure, and their excellent characteristics lay a solid foundation for electrocatalysis. This review systematically introduces the design principles of the catalytic sites in two-dimensional (2D) COF-based electrocatalysts and analyzes the relationship between 2D COF structure and their electrocatalytic performances. In particular, the recent progress in the field of 2D COFs as electrocatalysts is comprehensively summarized. Finally, we discuss the current shortcomings and challenges on tailoring 2D COF for high-performance electrocatalysts in details, and look forward to promoting more researches on 2D COF-based electrocatalysts.[Figure not available: see fulltext.].

KW - active centers

KW - covalent organic frameworks

KW - electrocatalysts

KW - two-dimensional

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SP - 8570

EP - 8595

JO - Nano Research

JF - Nano Research

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ER -

Two-dimensional covalent organic frameworks for electrocatalysis: Achievements, challenges, and opportunities

Abstract

Keywords

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