TY - JOUR
T1 - Transition path dynamics across rough inverted parabolic potential barrier
AU - Li, Hua
AU - Xu, Yong
AU - Li, Yongge
AU - Metzler, Ralf
N1 - Publisher Copyright:
© 2020, Società Italiana di Fisica and Springer-Verlag GmbH Germany, part of Springer Nature.
PY - 2020/9/1
Y1 - 2020/9/1
N2 - Transition path dynamics have been widely studied in chemical, physical, and technological systems. Mostly, the transition path dynamics is obtained for smooth barrier potentials, for instance, generic inverse-parabolic shapes. We here present analytical results for the mean transition path time, the distribution of transition path times, the mean transition path velocity, and the mean transition path shape in a rough inverted parabolic potential function under the driving of Gaussian white noise. These are validated against extensive simulations using the forward flux sampling scheme in parallel computations. We observe how precisely the potential roughness, the barrier height, and the noise intensity contribute to the particle transition in the rough inverted barrier potential.
AB - Transition path dynamics have been widely studied in chemical, physical, and technological systems. Mostly, the transition path dynamics is obtained for smooth barrier potentials, for instance, generic inverse-parabolic shapes. We here present analytical results for the mean transition path time, the distribution of transition path times, the mean transition path velocity, and the mean transition path shape in a rough inverted parabolic potential function under the driving of Gaussian white noise. These are validated against extensive simulations using the forward flux sampling scheme in parallel computations. We observe how precisely the potential roughness, the barrier height, and the noise intensity contribute to the particle transition in the rough inverted barrier potential.
UR - http://www.scopus.com/inward/record.url?scp=85090950464&partnerID=8YFLogxK
U2 - 10.1140/epjp/s13360-020-00752-7
DO - 10.1140/epjp/s13360-020-00752-7
M3 - 文章
AN - SCOPUS:85090950464
SN - 2190-5444
VL - 135
JO - European Physical Journal Plus
JF - European Physical Journal Plus
IS - 9
M1 - 731
ER -