TY - JOUR
T1 - Shear Evolution and Slippage of the Liquid-Liquid Interface over a Liquid-Infused Surface
T2 - A Many-Body Dissipative Particle Dynamics Study
AU - Ren, Liuzhen
AU - Ren, Jiangzhuo
AU - Bao, Luyao
AU - Wen, Jun
AU - Ye, Min
AU - Hu, Haibao
N1 - Publisher Copyright:
© 2025 American Chemical Society.
PY - 2025/3/4
Y1 - 2025/3/4
N2 - The liquid-liquid interface (LLI), which is the key to cause flow slippage and thus promote drag reduction of liquid-infused surfaces (LISs), does suffer from the action of flow shear. In the current study, the transverse many-body dissipative dynamics simulation method is applied to explore the shear evolution of LLI and the corresponding slippage over a periodically grooved LIS. Results show that a relatively small shear rate only induces a slight deformation of LLI and the corresponding effective slippage is dependent on the shear rate. With a further increase of the shear rate, LLI deforms apparently and then the downstream three phase contact line depins to move once the balance between the capillary force and the shear force is broken, which results in an apparent increase of the slippage, specifically for a convex LLI. Compared with a convex LLI or a concave LLI, a flat LLI remains relatively stable under the same shear action, and an increase of the viscosity ratio and a decrease of the LLI fraction can both strengthen the shear resistance of an LLI, while they are less effective to promote the slippage. Consequently, the current results not only indicate that the slippage is related to the interface deflection and the shear rate but also suggest that both the shear resistance and the slippage of LLI should be considered when designing an effective LIS.
AB - The liquid-liquid interface (LLI), which is the key to cause flow slippage and thus promote drag reduction of liquid-infused surfaces (LISs), does suffer from the action of flow shear. In the current study, the transverse many-body dissipative dynamics simulation method is applied to explore the shear evolution of LLI and the corresponding slippage over a periodically grooved LIS. Results show that a relatively small shear rate only induces a slight deformation of LLI and the corresponding effective slippage is dependent on the shear rate. With a further increase of the shear rate, LLI deforms apparently and then the downstream three phase contact line depins to move once the balance between the capillary force and the shear force is broken, which results in an apparent increase of the slippage, specifically for a convex LLI. Compared with a convex LLI or a concave LLI, a flat LLI remains relatively stable under the same shear action, and an increase of the viscosity ratio and a decrease of the LLI fraction can both strengthen the shear resistance of an LLI, while they are less effective to promote the slippage. Consequently, the current results not only indicate that the slippage is related to the interface deflection and the shear rate but also suggest that both the shear resistance and the slippage of LLI should be considered when designing an effective LIS.
UR - http://www.scopus.com/inward/record.url?scp=86000377452&partnerID=8YFLogxK
U2 - 10.1021/acs.langmuir.4c04428
DO - 10.1021/acs.langmuir.4c04428
M3 - 文章
AN - SCOPUS:86000377452
SN - 0743-7463
VL - 41
SP - 5158
EP - 5169
JO - Langmuir
JF - Langmuir
IS - 8
ER -