TY - JOUR
T1 - Ion migration controlled stability in α particle response of cspbbr2.4cl0.6 detectors
AU - Zhang, Bin Bin
AU - Wang, Fangbao
AU - Liu, Xin
AU - Xiao, Bao
AU - Xu, Meng
AU - Dong, Song Tao
AU - Xu, Yadong
AU - Sellin, Paul
AU - Jie, Wanqi
N1 - Publisher Copyright:
© 2021 American Chemical Society. All rights reserved.
PY - 2021/2/25
Y1 - 2021/2/25
N2 - Halide perovskites have been considered as nuclear radiation detection materials due to their high mobility, long carrier lifetime, and high absorption coefficient. However, it has been reported that the ion migration increases the dark current of halide perovskite detectors and hinders the stable response to high energy photons or particles. In this work, we report the utilization of the "voltage cycling" technique to obtain the stable α-particle spectra in a CsPbBr2.4Cl0.6 device. Also, by measuring the timedependent stability and the effect of electric field strength, we can gain insight into the phenomona causing instability in these devices. Accordingly, the influence of ion migration on the charge transport properties and energy spectra in CsPbBr2.4Cl0.6 detectors was also revealed. Our investigation demonstrates the strong correlation between ion migration processes and stable energy spectra in halide perovskite materials.
AB - Halide perovskites have been considered as nuclear radiation detection materials due to their high mobility, long carrier lifetime, and high absorption coefficient. However, it has been reported that the ion migration increases the dark current of halide perovskite detectors and hinders the stable response to high energy photons or particles. In this work, we report the utilization of the "voltage cycling" technique to obtain the stable α-particle spectra in a CsPbBr2.4Cl0.6 device. Also, by measuring the timedependent stability and the effect of electric field strength, we can gain insight into the phenomona causing instability in these devices. Accordingly, the influence of ion migration on the charge transport properties and energy spectra in CsPbBr2.4Cl0.6 detectors was also revealed. Our investigation demonstrates the strong correlation between ion migration processes and stable energy spectra in halide perovskite materials.
UR - http://www.scopus.com/inward/record.url?scp=85101506719&partnerID=8YFLogxK
U2 - 10.1021/acs.jpcc.0c10758
DO - 10.1021/acs.jpcc.0c10758
M3 - 文章
AN - SCOPUS:85101506719
SN - 1932-7447
VL - 125
SP - 4235
EP - 4242
JO - Journal of Physical Chemistry C
JF - Journal of Physical Chemistry C
IS - 7
ER -