Hydrothermal synthesis, crystal structure and electrochemical behavior of 2D hybrid coordination polymer

Weiqiang Fan, Lin Zhu, Weidong Shi, Fuxiao Chen, Hongye Bai, Shuyan Song, Yongsheng Yan

Research output: Contribution to journalArticlepeer-review

3 Scopus citations

Abstract

A novel metal-organic coordination polymer [Cu(phen)(L) 0.5(H2O)]n (H4L = (N,N′-5,5′-bis(isophthalic acid)-p-xylylenediamine, and phen = 1,10-phenanthroline) has been hydrothermally synthesized and characterized by elemental analysis, IR, TGA, and single-crystal X-ray diffraction. The crystallographic data show that the title compound crystallizes in monoclinic space group P21/n with a = 10.682(2), b = 15.682(3), c = 11.909(2) Å, β = 91.39(3)°, V = 1994.3(7) Å3, C 24H17CuN3O5, Mr = 490.95, Dc = 1.635 g/cm3, F(000) = 1004, Z = 4, μ(MoKα) = 1.141 mm-1, the final R = 0.0418 and wR = 0.0983 for 3578 observed reflections (I > 2σ(I)). The structural analyses reveal that the title compound exhibits shows a 2D layer structure, which are further linked by hydrogen bonding interactions to form a three-dimensional supramolecular network. In addition, the thermal stability and electrochemical behavior of title compound has been studied. CCDC: 900413.

Original languageEnglish
Article number1350027
JournalFunctional Materials Letters
Volume6
Issue number3
DOIs
StatePublished - Jun 2013
Externally publishedYes

Keywords

  • crystal structure
  • electrochemical behavior
  • Hydrothermal synthesis

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