TY - JOUR
T1 - Analysis of spatiotemporal variation of formaldehyde column concentration in Qinghai-Tibet Plateau and its influencing factors
AU - Zhang, Yongjia
AU - Ju, Tianzhen
AU - Shi, Yao
AU - Wang, Qing Qing
AU - Li, Feng Shuai
AU - Zhang, Guoqiang
N1 - Publisher Copyright:
© 2021, The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.
PY - 2021/10
Y1 - 2021/10
N2 - Based on the formaldehyde (HCHO) inversion data of OMI satellite sensor from 2009 to 2019, this paper discusses the spatial and temporal distribution of HCHO column concentration over the Qinghai-Tibet Plateau in the past 11 years and explores the factors affecting the dynamic distribution of atmospheric HCHO column concentration over the Qinghai-Tibet Plateau in combination with meteorological, aerosol, ozone, and other data. The results show that the average concentration of HCHO column in the Qinghai-Tibet Plateau is 8.84 × 1015 molec/cm2 in the past 11 years, which is relatively low, and the annual variation rate of HCHO column is 7.79%, showing a slight upward trend. The seasonal changes show a trend of Autumn < Winter < Spring < Summer. The monthly variation is more obvious than the seasonal variation. The spatial distribution showed a decreasing trend from southeast to northwest. Residual analysis showed that 83.77% of the area was frequently affected by natural factors. Correlation analysis found that the natural factors including precipitation, air temperature, and atmospheric activities for a greater influence on the column experiment the distribution of the concentration of the Qinghai-Tibet Plateau and human factors, such as biomass, the distribution of fossil fuel combustion, and emissions to HCHO, play a promoting role. Through the backward trajectory analysis, it can be seen that the transboundary atmospheric transport activity has a prominent contribution to the distribution of HCHO in the southern region of the Qinghai-Tibet Plateau. Hurst index study found that in the future, the concentration of HCHO column in 53.03% of the Qinghai-Tibet Plateau will decrease, but in some areas, such as the eastern and northern parts of the Qinghai-Tibet Plateau, it will increase.
AB - Based on the formaldehyde (HCHO) inversion data of OMI satellite sensor from 2009 to 2019, this paper discusses the spatial and temporal distribution of HCHO column concentration over the Qinghai-Tibet Plateau in the past 11 years and explores the factors affecting the dynamic distribution of atmospheric HCHO column concentration over the Qinghai-Tibet Plateau in combination with meteorological, aerosol, ozone, and other data. The results show that the average concentration of HCHO column in the Qinghai-Tibet Plateau is 8.84 × 1015 molec/cm2 in the past 11 years, which is relatively low, and the annual variation rate of HCHO column is 7.79%, showing a slight upward trend. The seasonal changes show a trend of Autumn < Winter < Spring < Summer. The monthly variation is more obvious than the seasonal variation. The spatial distribution showed a decreasing trend from southeast to northwest. Residual analysis showed that 83.77% of the area was frequently affected by natural factors. Correlation analysis found that the natural factors including precipitation, air temperature, and atmospheric activities for a greater influence on the column experiment the distribution of the concentration of the Qinghai-Tibet Plateau and human factors, such as biomass, the distribution of fossil fuel combustion, and emissions to HCHO, play a promoting role. Through the backward trajectory analysis, it can be seen that the transboundary atmospheric transport activity has a prominent contribution to the distribution of HCHO in the southern region of the Qinghai-Tibet Plateau. Hurst index study found that in the future, the concentration of HCHO column in 53.03% of the Qinghai-Tibet Plateau will decrease, but in some areas, such as the eastern and northern parts of the Qinghai-Tibet Plateau, it will increase.
KW - Backward trajectory
KW - HCHO column concentration
KW - Influencing factors
KW - OMI
KW - Qinghai-Tibet Plateau
UR - http://www.scopus.com/inward/record.url?scp=85107942068&partnerID=8YFLogxK
U2 - 10.1007/s11356-021-14719-3
DO - 10.1007/s11356-021-14719-3
M3 - 文章
C2 - 34129162
AN - SCOPUS:85107942068
SN - 0944-1344
VL - 28
SP - 55233
EP - 55251
JO - Environmental Science and Pollution Research
JF - Environmental Science and Pollution Research
IS - 39
ER -