TY - JOUR
T1 - Plasmon-enhanced photoluminescence from TiO2:Sm3+:Au nanostructure
AU - An, Guofei
AU - Yang, Chaoshun
AU - Zhou, Yawei
AU - Zhao, Xiaopeng
PY - 2012/12
Y1 - 2012/12
N2 - In this paper, a novel plasmon-enhanced photoluminescence (PL) hybrid system is presented based on metal-semiconductor nanostructure, in which TiO2:Sm3+ works as luminophor while the gold nanoparticle (NP) as the promoter of plasmon resonance. The plasmon-enhanced PL is obtained by optimizing the plasmon resonance peak of gold NP employed in the system, and it is deduced that there is energy transfer from TiO2:Sm3+ to Au NPs during the process of light emitting. When the localized surface plasmon resonance (LSPR) spectra of Au NPs overlap with the PL spectra of TiO2:Sm3+, the Au NPs absorb the energy transferred from TiO2:Sm3+, and then the plasmonic mode confined around Au NPs can be excited to bring out the PL enhancement. Schematic illustration of the process of plasmon-enhanced emission. The different steps are (a) light emitting of TiO2:Sm3+, (b) energy transferred from TiO2:Sm3+ to the Au NPs, and (c) enhanced emitting of the hybrid system.
AB - In this paper, a novel plasmon-enhanced photoluminescence (PL) hybrid system is presented based on metal-semiconductor nanostructure, in which TiO2:Sm3+ works as luminophor while the gold nanoparticle (NP) as the promoter of plasmon resonance. The plasmon-enhanced PL is obtained by optimizing the plasmon resonance peak of gold NP employed in the system, and it is deduced that there is energy transfer from TiO2:Sm3+ to Au NPs during the process of light emitting. When the localized surface plasmon resonance (LSPR) spectra of Au NPs overlap with the PL spectra of TiO2:Sm3+, the Au NPs absorb the energy transferred from TiO2:Sm3+, and then the plasmonic mode confined around Au NPs can be excited to bring out the PL enhancement. Schematic illustration of the process of plasmon-enhanced emission. The different steps are (a) light emitting of TiO2:Sm3+, (b) energy transferred from TiO2:Sm3+ to the Au NPs, and (c) enhanced emitting of the hybrid system.
KW - gold nanoparticle
KW - luminescence enhancement
KW - rare-earth doping
KW - TiO
UR - http://www.scopus.com/inward/record.url?scp=84871252912&partnerID=8YFLogxK
U2 - 10.1002/pssa.201228290
DO - 10.1002/pssa.201228290
M3 - 文章
AN - SCOPUS:84871252912
SN - 1862-6300
VL - 209
SP - 2583
EP - 2588
JO - Physica Status Solidi (A) Applications and Materials Science
JF - Physica Status Solidi (A) Applications and Materials Science
IS - 12
ER -