Highly stable water-soluble ZnSe:Cu quantum dots coated with doubly ZnS shell

Xiaoyan Li, Chaojin Xuan, Boxu Yang, Weichen Wang, Mingzhong Wang, Xiaopeng Zhao

科研成果: 期刊稿件文章同行评审

6 引用 (Scopus)

摘要

Doped ZnSe quantum dots (QDs) have become a potential substitute for Cd-based QDs. In this paper, center-doped monodisperse Cu-doped ZnSe (ZnSe:Cu) QDs are synthesized as the first step in aqueous solution by co-nucleation doping method, and then the double-layered ZnS shell is grown by successive growth. The prepared ZnSe:Cu/ZnS/ZnS QDs have high photoluminescence(PL) intensity and excellent stability in the blue region. The crystal structure has not been changed and the PL intensity maintains 95% after 365 days stored in the air. The outstanding performance of the prepared QDs benefit from the ZnS shell grown outside the core of ZnSe:Cu, especially the second layer of the ZnS shell can effectively limit excitons and Cu in the ZnSe core and isolate O2. The strategy in our work paves a new path to elevate the stability of QDs.

源语言英语
文章编号169406
期刊Journal of Alloys and Compounds
947
DOI
出版状态已出版 - 25 6月 2023

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