Fabrication of folded MXene/MoS₂ composite microspheres with optimal composition and their microwave absorbing properties

In this work, ultrasonic spray technology is utilized for build up MXene and MoS₂ nanosheets to three-dimensional MXene/MoS₂ fold microspheres by one-step method. By skillfully assembling two kinds of functional two-dimensional materials, the microspheres have abundant heterogeneous interfaces and huge specific surface area. The optimum feed ratio of MXene and MoS₂ is determined by comparing the absorbing properties, and the mass ratio is 5:1. With 30% filler, the material shows the best absorption performance. At 10.4 GHz, the minimal reflection loss (RL_min) reach −51.21 dB, and the thickness is merely 2.5 mm. At the thickness in 1.6 mm, the efficacious absorption bandwidth (RL < -10 dB) reaches 4.4 GHz. The outstanding microwave absorbing properties with MXene/MoS₂ folded microspheres is resulted in the multiple interfaces in the heterostructure and above the average conductivity of MXene. The results show that MXene/MoS₂ folded microsphere is a prospective electromagnetic absorbing material. The construction of MXene/MoS₂ folded microsphere provides an effective method to devise new high-performance microwave absorbing materials.