TY - JOUR
T1 - Emerging Trends in Sustainable CO2-Management Materials
AU - Zhang, Zhen
AU - Zheng, Yun
AU - Qian, Lanting
AU - Luo, Dan
AU - Dou, Haozhen
AU - Wen, Guobin
AU - Yu, Aiping
AU - Chen, Zhongwei
N1 - Publisher Copyright:
© 2022 Wiley-VCH GmbH.
PY - 2022/7/21
Y1 - 2022/7/21
N2 - With the rising level of atmospheric CO2 worsening climate change, a promising global movement toward carbon neutrality is forming. Sustainable CO2 management based on carbon capture and utilization (CCU) has garnered considerable interest due to its critical role in resolving emission-control and energy-supply challenges. Here, a comprehensive review is presented that summarizes the state-of-the-art progress in developing promising materials for sustainable CO2 management in terms of not only capture, catalytic conversion (thermochemistry, electrochemistry, photochemistry, and possible combinations), and direct utilization, but also emerging integrated capture and in situ conversion as well as artificial-intelligence-driven smart material study. In particular, insights that span multiple scopes of material research are offered, ranging from mechanistic comprehension of reactions, rational design and precise manipulation of key materials (e.g., carbon nanomaterials, metal–organic frameworks, covalent organic frameworks, zeolites, ionic liquids), to industrial implementation. This review concludes with a summary and new perspectives, especially from multiple aspects of society, which summarizes major difficulties and future potential for implementing advanced materials and technologies in sustainable CO2 management. This work may serve as a guideline and road map for developing CCU material systems, benefiting both scientists and engineers working in this growing and potentially game-changing area.
AB - With the rising level of atmospheric CO2 worsening climate change, a promising global movement toward carbon neutrality is forming. Sustainable CO2 management based on carbon capture and utilization (CCU) has garnered considerable interest due to its critical role in resolving emission-control and energy-supply challenges. Here, a comprehensive review is presented that summarizes the state-of-the-art progress in developing promising materials for sustainable CO2 management in terms of not only capture, catalytic conversion (thermochemistry, electrochemistry, photochemistry, and possible combinations), and direct utilization, but also emerging integrated capture and in situ conversion as well as artificial-intelligence-driven smart material study. In particular, insights that span multiple scopes of material research are offered, ranging from mechanistic comprehension of reactions, rational design and precise manipulation of key materials (e.g., carbon nanomaterials, metal–organic frameworks, covalent organic frameworks, zeolites, ionic liquids), to industrial implementation. This review concludes with a summary and new perspectives, especially from multiple aspects of society, which summarizes major difficulties and future potential for implementing advanced materials and technologies in sustainable CO2 management. This work may serve as a guideline and road map for developing CCU material systems, benefiting both scientists and engineers working in this growing and potentially game-changing area.
KW - carbon capture and utilization
KW - CO management
KW - dual-functional materials
KW - energy sustainability
KW - smart materials
UR - http://www.scopus.com/inward/record.url?scp=85131823561&partnerID=8YFLogxK
U2 - 10.1002/adma.202201547
DO - 10.1002/adma.202201547
M3 - 文献综述
C2 - 35307897
AN - SCOPUS:85131823561
SN - 0935-9648
VL - 34
JO - Advanced Materials
JF - Advanced Materials
IS - 29
M1 - 2201547
ER -