Charge-State Control of a Host Metal-Organic Framework Enabled by Axially Coordinated Tripyridine Ligand Alternation

Tao Zhang; Jian Wei Cao; Yi Fei Dai; He Feng; Shu Yi Zhang; Juan Chen; Teng Wang; Yu Wang; Kai Jie Chen

doi:10.1021/acs.cgd.2c00403

Charge-State Control of a Host Metal-Organic Framework Enabled by Axially Coordinated Tripyridine Ligand Alternation

Tao Zhang, Jian Wei Cao, Yi Fei Dai, He Feng, Shu Yi Zhang, Juan Chen, Teng Wang, Yu Wang, Kai Jie Chen

化学与化工学院

科研成果: 期刊稿件 › 文章 › 同行评审

4 引用（Scopus）

摘要

Herein we demonstrate the charge-state control of a host framework by alternating the coordinating ligands in two isostructural metal-organic frameworks based on [Mn₃(μ₃-O)] clusters. The different charge states of two host frameworks were verified by multiple characterization techniques, altered methylene blue adsorption behavior and density functional theory calculations. The contribution of this study will provide useful guidelines for the future design of ionic coordination frameworks.

源语言	英语
页（从-至）	3594-3600
页数	7
期刊	Crystal Growth and Design
卷	22
期	6
DOI	https://doi.org/10.1021/acs.cgd.2c00403
出版状态	已出版 - 1 6月 2022

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10.1021/acs.cgd.2c00403

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abstract = "Herein we demonstrate the charge-state control of a host framework by alternating the coordinating ligands in two isostructural metal-organic frameworks based on [Mn3(μ3-O)] clusters. The different charge states of two host frameworks were verified by multiple characterization techniques, altered methylene blue adsorption behavior and density functional theory calculations. The contribution of this study will provide useful guidelines for the future design of ionic coordination frameworks.",

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T1 - Charge-State Control of a Host Metal-Organic Framework Enabled by Axially Coordinated Tripyridine Ligand Alternation

AU - Zhang, Tao

AU - Cao, Jian Wei

AU - Dai, Yi Fei

AU - Feng, He

AU - Zhang, Shu Yi

AU - Chen, Juan

AU - Wang, Teng

AU - Wang, Yu

AU - Chen, Kai Jie

PY - 2022/6/1

Y1 - 2022/6/1

N2 - Herein we demonstrate the charge-state control of a host framework by alternating the coordinating ligands in two isostructural metal-organic frameworks based on [Mn3(μ3-O)] clusters. The different charge states of two host frameworks were verified by multiple characterization techniques, altered methylene blue adsorption behavior and density functional theory calculations. The contribution of this study will provide useful guidelines for the future design of ionic coordination frameworks.

AB - Herein we demonstrate the charge-state control of a host framework by alternating the coordinating ligands in two isostructural metal-organic frameworks based on [Mn3(μ3-O)] clusters. The different charge states of two host frameworks were verified by multiple characterization techniques, altered methylene blue adsorption behavior and density functional theory calculations. The contribution of this study will provide useful guidelines for the future design of ionic coordination frameworks.

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U2 - 10.1021/acs.cgd.2c00403

DO - 10.1021/acs.cgd.2c00403

M3 - 文章

AN - SCOPUS:85131803974

SN - 1528-7483

VL - 22

SP - 3594

EP - 3600

JO - Crystal Growth and Design

JF - Crystal Growth and Design

IS - 6

ER -

Charge-State Control of a Host Metal-Organic Framework Enabled by Axially Coordinated Tripyridine Ligand Alternation

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