Texture Regulation of Metal–Organic Frameworks, Microwave Absorption Mechanism-Oriented Structural Optimization and Design Perspectives

Zhenguo Gao, Aamir Iqbal, Tufail Hassan, Limin Zhang, Hongjing Wu, Chong Min Koo

Research output: Contribution to journalReview articlepeer-review

125 Scopus citations

Abstract

Texture regulation of metal–organic frameworks (MOFs) is essential for controlling their electromagnetic wave (EMW) absorption properties. This review systematically summarizes the recent advancements in texture regulation strategies for MOFs, including etching and exchange of central ions, etching and exchange of ligands, chemically induced self-assembly, and MOF-on-MOF heterostructure design. Additionally, the EMW absorption mechanisms in approaches based on structure–function dependencies, including nano-micro topological engineering, defect engineering, interface engineering, and hybrid engineering, are comprehensively explored. Finally, current challenges and future research orientation are proposed. This review aims to provide new perspectives for designing MOF-derived EMW-absorption materials to achieve essential breakthroughs in mechanistic investigations in this promising field.

Original languageEnglish
Article number2204151
JournalAdvanced Science
Volume9
Issue number35
DOIs
StatePublished - 19 Dec 2022

Keywords

  • electromagnetic wave absorption
  • metal–organic frameworks (MOFs)
  • optimization engineering
  • texture regulation

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