Studying of Co-doped g-C3N4 and modified with Fe3O4 quantum dots on removing tetracycline

Zhi Zhu, Xu Tang, Wenqian Fan, Zhi Liu, Pengwei Huo, Tianshuai Wang, Yongsheng Yan, Chunxiang Li

Research output: Contribution to journalArticlepeer-review

53 Scopus citations

Abstract

A new Co-doped and Fe3O4 quantum dots (QDs) decorated g-C3N4 (CN) photocatalyst applied in the tetracycline degradation under visible light irradiation, is designed and synthesized. The Fe3O4-QDs@Co–CN enhanced photocatalytic activity and cycling ability in comparison with individual CN significantly. It revealed a synergistic effect between the formation of Fe3O4-QDs and Co-doping. Results of characterization insight into the reason that Co-doped can regulate the band gap of CN, which has been proved by XPS and density functional theory (DFT). Moreover, the oxidation-reduction centre of Fe3O4-QDs with quantum effect can significantly boost the absorption of visible light and utilization electrons. Therefore, this work provides a broadening window for photo harvesting, charge using and separation during photocatalytic reactions.

Original languageEnglish
Pages (from-to)248-258
Number of pages11
JournalJournal of Alloys and Compounds
Volume775
DOIs
StatePublished - 15 Feb 2019
Externally publishedYes

Keywords

  • Co-doped
  • Density functional theory
  • FeO-QDs
  • Oxidation-reduction centre
  • Photocatalytic degradation
  • Quantum effect

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