Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol

Ruilong Zhang; Zhiping Zhou; Atian Xie; Jiangdong Dai; Jiuyun Cui; Jihui Lang; Maobin Wei; Xiaohui Dai; Chunxiang Li; Yongsheng Yan

doi:10.1016/j.jtice.2017.07.032

Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol

Ruilong Zhang, Zhiping Zhou, Atian Xie, Jiangdong Dai, Jiuyun Cui, Jihui Lang, Maobin Wei, Xiaohui Dai, Chunxiang Li, Yongsheng Yan

Research output: Contribution to journal › Article › peer-review

26 Scopus citations

Abstract

The wide applications of antibiotics in human and veterinary medicines have attracted ever-increasing attention due to their potential adverse effects for ecological environment, therefore, it is urgent and important to efficiently remove antibiotics from water. In this paper, we prepared hierarchical porous carbons from sodium carboxymethyl cellulose (CMCHPCs) via halloysite template and KOH-activation method for efficient removal of chloramphenicol. The physicochemical properties of CMCHPCs are analyzed by means of different characterizations. The adsorption properties of CMCHPCs are evaluated by equilibrium, kinetic, and thermodynamic adsorption experiments. In addition, the effects of ionic strength, solution pH, and humic acid on adsorption are studied. The results indicated CMCHPCs exhibit higher maximum monolayer adsorption capacity up to 769.95 mg/g and shows good regenerability and adaptability. Importantly, the adsorption mechanisms of chloramphenicol adsorbed onto the CMCHPCs are also discussed.

Original language	English
Pages (from-to)	424-433
Number of pages	10
Journal	Journal of the Taiwan Institute of Chemical Engineers
Volume	80
DOIs	https://doi.org/10.1016/j.jtice.2017.07.032
State	Published - Nov 2017
Externally published	Yes

Keywords

Antibiotics removal
Biomass
Halloysite template
Hierarchical porous carbon materials
KOH-activation

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1016/j.jtice.2017.07.032

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Zhang, R., Zhou, Z., Xie, A., Dai, J., Cui, J., Lang, J., Wei, M., Dai, X., Li, C., & Yan, Y. (2017). Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol. Journal of the Taiwan Institute of Chemical Engineers, 80, 424-433. https://doi.org/10.1016/j.jtice.2017.07.032

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title = "Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol",

abstract = "The wide applications of antibiotics in human and veterinary medicines have attracted ever-increasing attention due to their potential adverse effects for ecological environment, therefore, it is urgent and important to efficiently remove antibiotics from water. In this paper, we prepared hierarchical porous carbons from sodium carboxymethyl cellulose (CMCHPCs) via halloysite template and KOH-activation method for efficient removal of chloramphenicol. The physicochemical properties of CMCHPCs are analyzed by means of different characterizations. The adsorption properties of CMCHPCs are evaluated by equilibrium, kinetic, and thermodynamic adsorption experiments. In addition, the effects of ionic strength, solution pH, and humic acid on adsorption are studied. The results indicated CMCHPCs exhibit higher maximum monolayer adsorption capacity up to 769.95 mg/g and shows good regenerability and adaptability. Importantly, the adsorption mechanisms of chloramphenicol adsorbed onto the CMCHPCs are also discussed.",

keywords = "Antibiotics removal, Biomass, Halloysite template, Hierarchical porous carbon materials, KOH-activation",

author = "Ruilong Zhang and Zhiping Zhou and Atian Xie and Jiangdong Dai and Jiuyun Cui and Jihui Lang and Maobin Wei and Xiaohui Dai and Chunxiang Li and Yongsheng Yan",

note = "Publisher Copyright: {\textcopyright} 2017 Taiwan Institute of Chemical Engineers",

year = "2017",

month = nov,

doi = "10.1016/j.jtice.2017.07.032",

language = "英语",

volume = "80",

pages = "424--433",

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Zhang, R, Zhou, Z, Xie, A, Dai, J, Cui, J, Lang, J, Wei, M, Dai, X, Li, C & Yan, Y 2017, 'Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol', Journal of the Taiwan Institute of Chemical Engineers, vol. 80, pp. 424-433. https://doi.org/10.1016/j.jtice.2017.07.032

Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol. / Zhang, Ruilong; Zhou, Zhiping; Xie, Atian et al.
In: Journal of the Taiwan Institute of Chemical Engineers, Vol. 80, 11.2017, p. 424-433.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol

AU - Zhang, Ruilong

AU - Zhou, Zhiping

AU - Xie, Atian

AU - Dai, Jiangdong

AU - Cui, Jiuyun

AU - Lang, Jihui

AU - Wei, Maobin

AU - Dai, Xiaohui

AU - Li, Chunxiang

AU - Yan, Yongsheng

PY - 2017/11

Y1 - 2017/11

N2 - The wide applications of antibiotics in human and veterinary medicines have attracted ever-increasing attention due to their potential adverse effects for ecological environment, therefore, it is urgent and important to efficiently remove antibiotics from water. In this paper, we prepared hierarchical porous carbons from sodium carboxymethyl cellulose (CMCHPCs) via halloysite template and KOH-activation method for efficient removal of chloramphenicol. The physicochemical properties of CMCHPCs are analyzed by means of different characterizations. The adsorption properties of CMCHPCs are evaluated by equilibrium, kinetic, and thermodynamic adsorption experiments. In addition, the effects of ionic strength, solution pH, and humic acid on adsorption are studied. The results indicated CMCHPCs exhibit higher maximum monolayer adsorption capacity up to 769.95 mg/g and shows good regenerability and adaptability. Importantly, the adsorption mechanisms of chloramphenicol adsorbed onto the CMCHPCs are also discussed.

AB - The wide applications of antibiotics in human and veterinary medicines have attracted ever-increasing attention due to their potential adverse effects for ecological environment, therefore, it is urgent and important to efficiently remove antibiotics from water. In this paper, we prepared hierarchical porous carbons from sodium carboxymethyl cellulose (CMCHPCs) via halloysite template and KOH-activation method for efficient removal of chloramphenicol. The physicochemical properties of CMCHPCs are analyzed by means of different characterizations. The adsorption properties of CMCHPCs are evaluated by equilibrium, kinetic, and thermodynamic adsorption experiments. In addition, the effects of ionic strength, solution pH, and humic acid on adsorption are studied. The results indicated CMCHPCs exhibit higher maximum monolayer adsorption capacity up to 769.95 mg/g and shows good regenerability and adaptability. Importantly, the adsorption mechanisms of chloramphenicol adsorbed onto the CMCHPCs are also discussed.

KW - Antibiotics removal

KW - Biomass

KW - Halloysite template

KW - Hierarchical porous carbon materials

KW - KOH-activation

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U2 - 10.1016/j.jtice.2017.07.032

DO - 10.1016/j.jtice.2017.07.032

M3 - 文章

AN - SCOPUS:85027249117

SN - 1876-1070

VL - 80

SP - 424

EP - 433

JO - Journal of the Taiwan Institute of Chemical Engineers

JF - Journal of the Taiwan Institute of Chemical Engineers

ER -

Preparation of hierarchical porous carbons from sodium carboxymethyl cellulose via halloysite template strategy coupled with KOH-activation for efficient removal of chloramphenicol

Abstract

Keywords

UN SDGs

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