High magnetic field-induced structural transformation of NiFe2O4/Fe2O3 heterostructures for enhancing lithium storage performance

Jia qi LIU, Rong yuan ZHANG, Xiao yang WANG, Jun WANG, Tie LIU, Wei bin CUI, Qiang WANG, Shuang YUAN

Research output: Contribution to journalArticlepeer-review

Abstract

In response to the limitations of conventional chemical synthesis methods for the structural modulation of nanomaterials, an innovative high magnetic field-assisted wet chemical synthesis method was proposed to prepare NiFe2O4/Fe2O3 heterostructures. It is found that the high-energy physical field could induce a more homogeneous morphology of NiFe2O4/Fe2O3, accompanied by phase transformation from Fe2O3 to NiFe2O4. As a result, the optimized structure obtained under the magnetic field endows NiFe2O4/Fe2O3 with enhanced performance for the lithium-ion battery anode, as evidenced by an increase of 16% (1200 mA·h/g) in discharge capacity and 24% in ultra-stable cycling performance (capacity retention of 97.1%). These results highlight the feasibility of high magnetic fields in modulating material structure and enhancing lithium storage performance.

Original languageEnglish
Pages (from-to)932-944
Number of pages13
JournalTransactions of Nonferrous Metals Society of China (English Edition)
Volume35
Issue number3
DOIs
StatePublished - Mar 2025

Keywords

  • heterostructure
  • high magnetic field
  • lithium-ion battery anode
  • NiFeO/FeO
  • structural regulation

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