Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Wei Fang; Chengfeng Du; Min Kuang; Mengxin Chen; Wenjing Huang; Hao Ren; Jianwei Xu; Armin Feldhoff; Qingyu Yan

doi:10.1039/d0cc01759k

Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Wei Fang, Chengfeng Du, Min Kuang, Mengxin Chen, Wenjing Huang, Hao Ren, Jianwei Xu, Armin Feldhoff, Qingyu Yan

School of Materials Sience and Engineering

Research output: Contribution to journal › Article › peer-review

63 Scopus citations

Abstract

An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti₃C₂T_x, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h^-1mg_cat^-1(equivalent to 45.16 µmol h^-1g_cat^-1HNO₃) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

Original language	English
Pages (from-to)	5779-5782
Number of pages	4
Journal	Chemical Communications
Volume	56
Issue number	43
DOIs	https://doi.org/10.1039/d0cc01759k
State	Published - 28 May 2020

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title = "Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst",

abstract = "An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.",

author = "Wei Fang and Chengfeng Du and Min Kuang and Mengxin Chen and Wenjing Huang and Hao Ren and Jianwei Xu and Armin Feldhoff and Qingyu Yan",

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T1 - Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

AU - Fang, Wei

AU - Du, Chengfeng

AU - Kuang, Min

AU - Chen, Mengxin

AU - Huang, Wenjing

AU - Ren, Hao

AU - Xu, Jianwei

AU - Feldhoff, Armin

AU - Yan, Qingyu

PY - 2020/5/28

Y1 - 2020/5/28

N2 - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

AB - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

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U2 - 10.1039/d0cc01759k

DO - 10.1039/d0cc01759k

M3 - 文章

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AN - SCOPUS:85085598970

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VL - 56

SP - 5779

EP - 5782

JO - Chemical Communications

JF - Chemical Communications

IS - 43

ER -

Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

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