A novel dielectric barrier discharge reactor with photocatalytic electrode based on sintered metal fibers for abatement of xylene

Zhiping Ye, Chunxia Wang, Zhenhua Shao, Qing Ye, Yi He, Yao Shi

Research output: Contribution to journalArticlepeer-review

28 Scopus citations

Abstract

A novel dielectric barrier discharge (DBD) reactor was made for the abatement of xylene. This reactor has a photocatalytic electrode prepared by a modified anodic oxidation method which was proposed in this work. The photocatalytic electrode has nano-TiO2 deposited on sintered metal fiber (SMF). The reactor using the nano-TiO2/SMF electrode shows much better performance in abating xylene compared with reactors using other electrodes such as resistance wire or SMF. The conversion ratio of xylene reaches 92.7% in the novel reactor at a relatively voltage (23.6kV). This ratio is much higher than the conversion ratios of xylene in the traditional reactors with resistance wire or SMF electrodes, which are ∼64.7%. The selectivity of CO2 of the reactor using the nano-TiO2/SMF electrode (300pps, 23.6kV) was observed to be 86.6%, which is about twice as large as that of a traditional reactor using a resistance wire electrode. If a traditional DBD reactor is replaced by the novel reactor, at the same specific input energy, the energy yield can increase from 0.391 to 0.556mg/kJ. Finally, the xylene decomposition mechanism with the nano-TiO2/SMF electrode was also briefly discussed.

Original languageEnglish
Pages (from-to)216-223
Number of pages8
JournalJournal of Hazardous Materials
Volume241-242
DOIs
StatePublished - 30 Nov 2012
Externally publishedYes

Keywords

  • Anodic oxidation
  • Dielectric barrier discharge
  • Nano-TiO/SMF electrode
  • Ti
  • Xylene

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