TY - JOUR
T1 - A high-performance 75 W direct ammonia fuel cell stack
AU - Wang, Teng
AU - Zhao, Yun
AU - Setzler, Brian P.
AU - Abbasi, Reza
AU - Gottesfeld, Shimshon
AU - Yan, Yushan
N1 - Publisher Copyright:
© 2022 The Authors
PY - 2022/4/20
Y1 - 2022/4/20
N2 - The low-temperature direct ammonia fuel cell (DAFC) is an attractive option for zero-emission transportation. However, the demonstration of high-performance and durable DAFCs and the identification of their suitable market are not yet reported. Here, we show a high-performance DAFC enabled by a hydrophobic spinel cathode, which achieves peak power density of 410 mW cm−2 and continuous operation for 80 h at 300 mA cm−2. We assemble five 50 cm2 cells into a 75 W DAFC stack, showing a comparable area-specific performance to that of the single cell. The best combination of performance and durability for the single cell and, particularly, the demonstration of, to the best of our knowledge, the world's first DAFC bipolar stack constitute a significant development of DAFC technology. We also perform an in-depth techno-economic analysis of a 2 kW, 10 kWh DAFC system serving for drones. DAFC systems with the performance obtained herein could be a competitive power source alongside hydrogen fuel cells and Li-ion batteries.
AB - The low-temperature direct ammonia fuel cell (DAFC) is an attractive option for zero-emission transportation. However, the demonstration of high-performance and durable DAFCs and the identification of their suitable market are not yet reported. Here, we show a high-performance DAFC enabled by a hydrophobic spinel cathode, which achieves peak power density of 410 mW cm−2 and continuous operation for 80 h at 300 mA cm−2. We assemble five 50 cm2 cells into a 75 W DAFC stack, showing a comparable area-specific performance to that of the single cell. The best combination of performance and durability for the single cell and, particularly, the demonstration of, to the best of our knowledge, the world's first DAFC bipolar stack constitute a significant development of DAFC technology. We also perform an in-depth techno-economic analysis of a 2 kW, 10 kWh DAFC system serving for drones. DAFC systems with the performance obtained herein could be a competitive power source alongside hydrogen fuel cells and Li-ion batteries.
KW - ammonia-tolerant catalyst
KW - carbon-neutral fuel
KW - direct ammonia fuel cell
KW - high-performance direct ammonia fuel cell
KW - techno-economic analysis
UR - http://www.scopus.com/inward/record.url?scp=85128447173&partnerID=8YFLogxK
U2 - 10.1016/j.xcrp.2022.100829
DO - 10.1016/j.xcrp.2022.100829
M3 - 文章
AN - SCOPUS:85128447173
SN - 2666-3864
VL - 3
JO - Cell Reports Physical Science
JF - Cell Reports Physical Science
IS - 4
M1 - 100829
ER -