Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Wei Fang; Chengfeng Du; Min Kuang; Mengxin Chen; Wenjing Huang; Hao Ren; Jianwei Xu; Armin Feldhoff; Qingyu Yan

doi:10.1039/d0cc01759k

Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

Wei Fang
, Chengfeng Du
, Min Kuang
, Mengxin Chen
, Wenjing Huang
, Hao Ren
, Jianwei Xu
, Armin Feldhoff
, Qingyu Yan

材料学院

Nanyang Technological University
Agency for Science, Technology and Research, Singapore
Leibniz University Hannover

科研成果: 期刊稿件 › 文章 › 同行评审

74 引用（Scopus）

摘要

An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti₃C₂T_x, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h^-1mg_cat^-1(equivalent to 45.16 µmol h^-1g_cat^-1HNO₃) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

源语言	英语
页（从-至）	5779-5782
页数	4
期刊	Chemical Communications
卷	56
期	43
DOI	https://doi.org/10.1039/d0cc01759k
出版状态	已出版 - 28 5月 2020

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10.1039/d0cc01759k

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title = "Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst",

abstract = "An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34\% in a favorable neutral pH environment.",

author = "Wei Fang and Chengfeng Du and Min Kuang and Mengxin Chen and Wenjing Huang and Hao Ren and Jianwei Xu and Armin Feldhoff and Qingyu Yan",

note = "Publisher Copyright: {\textcopyright} The Royal Society of Chemistry 2020.",

year = "2020",

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doi = "10.1039/d0cc01759k",

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T1 - Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

AU - Fang, Wei

AU - Du, Chengfeng

AU - Kuang, Min

AU - Chen, Mengxin

AU - Huang, Wenjing

AU - Ren, Hao

AU - Xu, Jianwei

AU - Feldhoff, Armin

AU - Yan, Qingyu

PY - 2020/5/28

Y1 - 2020/5/28

N2 - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

AB - An electrochemical nitrogen oxidation approach has been realized experimentally by a Pd-decorated MXene (Ti3C2Tx, T = F and O) electrocatalyst under ambient conditions. The Pd-MXene catalyst can achieve a desirable nitrate yield rate of 2.80 µg h-1mgcat-1(equivalent to 45.16 µmol h-1gcat-1HNO3) as well as a high nitrate faradaic efficiency of 11.34% in a favorable neutral pH environment.

UR - https://www.scopus.com/pages/publications/85085598970

U2 - 10.1039/d0cc01759k

DO - 10.1039/d0cc01759k

M3 - 文章

C2 - 32322861

AN - SCOPUS:85085598970

SN - 1359-7345

VL - 56

SP - 5779

EP - 5782

JO - Chemical Communications

JF - Chemical Communications

IS - 43

ER -

Boosting efficient ambient nitrogen oxidation by a well-dispersed Pd on MXene electrocatalyst

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