Phase structure and piezoelectric properties of high Curie temperature BiYbO3-PbTiO3-BaTiO3 ceramics

Gao Feng; Hong Rongzi; Liu Jiaji; Li Zhen; Cheng Lihong; Tian Changsheng

doi:10.1016/j.jallcom.2008.07.116

Phase structure and piezoelectric properties of high Curie temperature BiYbO₃-PbTiO₃-BaTiO₃ ceramics

Gao Feng
, Hong Rongzi
, Liu Jiaji
, Li Zhen
, Cheng Lihong
, Tian Changsheng

School of Materials Sience and Engineering

Northwestern Polytechnical University Xian

Research output: Contribution to journal › Article › peer-review

36 Scopus citations

Abstract

Perovskite (1 - x)(0.1BiYbO₃-0.9PbTiO₃)-xBaTiO₃ (BYPT-BT) ceramics were prepared by the conventional processing. The effect of BaTiO₃ on the microstructure and piezoelectric properties was investigated. The results show that the perovskite phase and the Yb₂Ti₂O₇ pyrochlore phase are coexisting in the BYPT-BT ceramics. BaTiO₃ influences the lattice structure and Ba²⁺ will replace A-site ions of perovskite, which decreases the lattice constant ratio c/a, leading to the lattice distortion. With increasing BaTiO₃ content, the percentage of pyrochlore phase decreases, which resulted in the increase of the dielectric constant ε and the piezoelectric constant d₃₃. BYPT-BT ceramics with the high Curie temperatures of > 500 °C are obtained. And BYPT-BT₄ ceramics with 0.12 mol BaTiO₃ has the optimal piezoelectric properties, ε is 720, tan δ is 0.013, d₃₃ is 34 pC/N, T_C is 505 °C.

Original language	English
Pages (from-to)	619-623
Number of pages	5
Journal	Journal of Alloys and Compounds
Volume	475
Issue number	1-2
DOIs	https://doi.org/10.1016/j.jallcom.2008.07.116
State	Published - 5 May 2009

Keywords

Curie temperature
Electrical properties
Piezoelectric ceramics
Pyrochlore phase

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10.1016/j.jallcom.2008.07.116

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@article{a390aeef0358465284d9952231d1e3ff,

title = "Phase structure and piezoelectric properties of high Curie temperature BiYbO3-PbTiO3-BaTiO3 ceramics",

abstract = "Perovskite (1 - x)(0.1BiYbO3-0.9PbTiO3)-xBaTiO3 (BYPT-BT) ceramics were prepared by the conventional processing. The effect of BaTiO3 on the microstructure and piezoelectric properties was investigated. The results show that the perovskite phase and the Yb2Ti2O7 pyrochlore phase are coexisting in the BYPT-BT ceramics. BaTiO3 influences the lattice structure and Ba2+ will replace A-site ions of perovskite, which decreases the lattice constant ratio c/a, leading to the lattice distortion. With increasing BaTiO3 content, the percentage of pyrochlore phase decreases, which resulted in the increase of the dielectric constant ε and the piezoelectric constant d33. BYPT-BT ceramics with the high Curie temperatures of > 500 °C are obtained. And BYPT-BT4 ceramics with 0.12 mol BaTiO3 has the optimal piezoelectric properties, ε is 720, tan δ is 0.013, d33 is 34 pC/N, TC is 505 °C.",

keywords = "Curie temperature, Electrical properties, Piezoelectric ceramics, Pyrochlore phase",

author = "Gao Feng and Hong Rongzi and Liu Jiaji and Li Zhen and Cheng Lihong and Tian Changsheng",

year = "2009",

month = may,

day = "5",

doi = "10.1016/j.jallcom.2008.07.116",

language = "英语",

volume = "475",

pages = "619--623",

journal = "Journal of Alloys and Compounds",

issn = "0925-8388",

publisher = "Elsevier B.V.",

number = "1-2",

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TY - JOUR

T1 - Phase structure and piezoelectric properties of high Curie temperature BiYbO3-PbTiO3-BaTiO3 ceramics

AU - Feng, Gao

AU - Rongzi, Hong

AU - Jiaji, Liu

AU - Zhen, Li

AU - Lihong, Cheng

AU - Changsheng, Tian

PY - 2009/5/5

Y1 - 2009/5/5

N2 - Perovskite (1 - x)(0.1BiYbO3-0.9PbTiO3)-xBaTiO3 (BYPT-BT) ceramics were prepared by the conventional processing. The effect of BaTiO3 on the microstructure and piezoelectric properties was investigated. The results show that the perovskite phase and the Yb2Ti2O7 pyrochlore phase are coexisting in the BYPT-BT ceramics. BaTiO3 influences the lattice structure and Ba2+ will replace A-site ions of perovskite, which decreases the lattice constant ratio c/a, leading to the lattice distortion. With increasing BaTiO3 content, the percentage of pyrochlore phase decreases, which resulted in the increase of the dielectric constant ε and the piezoelectric constant d33. BYPT-BT ceramics with the high Curie temperatures of > 500 °C are obtained. And BYPT-BT4 ceramics with 0.12 mol BaTiO3 has the optimal piezoelectric properties, ε is 720, tan δ is 0.013, d33 is 34 pC/N, TC is 505 °C.

AB - Perovskite (1 - x)(0.1BiYbO3-0.9PbTiO3)-xBaTiO3 (BYPT-BT) ceramics were prepared by the conventional processing. The effect of BaTiO3 on the microstructure and piezoelectric properties was investigated. The results show that the perovskite phase and the Yb2Ti2O7 pyrochlore phase are coexisting in the BYPT-BT ceramics. BaTiO3 influences the lattice structure and Ba2+ will replace A-site ions of perovskite, which decreases the lattice constant ratio c/a, leading to the lattice distortion. With increasing BaTiO3 content, the percentage of pyrochlore phase decreases, which resulted in the increase of the dielectric constant ε and the piezoelectric constant d33. BYPT-BT ceramics with the high Curie temperatures of > 500 °C are obtained. And BYPT-BT4 ceramics with 0.12 mol BaTiO3 has the optimal piezoelectric properties, ε is 720, tan δ is 0.013, d33 is 34 pC/N, TC is 505 °C.

KW - Curie temperature

KW - Electrical properties

KW - Piezoelectric ceramics

KW - Pyrochlore phase

UR - https://www.scopus.com/pages/publications/63649090513

U2 - 10.1016/j.jallcom.2008.07.116

DO - 10.1016/j.jallcom.2008.07.116

M3 - 文章

AN - SCOPUS:63649090513

SN - 0925-8388

VL - 475

SP - 619

EP - 623

JO - Journal of Alloys and Compounds

JF - Journal of Alloys and Compounds

IS - 1-2

ER -

Phase structure and piezoelectric properties of high Curie temperature BiYbO₃-PbTiO₃-BaTiO₃ ceramics

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Keywords

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