Microstructure evolution and reaction mechanism of Pb(Zr1/2Ti1/2)O3-Pb(Zn1/3Nb2/3)O3–Pb(Ni1/3Nb2/3)O3 piezoelectric ceramics with plate-like PbTiO3 template

Leilei Li; Junting Liu; Shuyao Cao; Jie Xu; Changying Wu; Emilia Pawlikowska; Mikołaj Szafran; Feng Gao

doi:10.1016/j.ceramint.2020.08.154

Microstructure evolution and reaction mechanism of Pb(Zr_1/2Ti_1/2)O₃-Pb(Zn_1/3Nb_2/3)O₃–Pb(Ni_1/3Nb_2/3)O₃ piezoelectric ceramics with plate-like PbTiO₃ template

Leilei Li
, Junting Liu
, Shuyao Cao
, Jie Xu
, Changying Wu
, Emilia Pawlikowska
, Mikołaj Szafran
, Feng Gao

School of Materials Sience and Engineering

Northwestern Polytechnical University Xian
Warsaw University of Technology

Research output: Contribution to journal › Article › peer-review

18 Scopus citations

Abstract

0.83 Pb(Zr_1/2Ti_1/2)O₃-0.11Pb(Zn_1/3Nb_2/3)O₃-0.06Pb(Ni_1/3Nb_2/3)O₃ (PZNNT) samples with plate-like PbTiO₃ (PT) template were prepared using tape casting technology. The microstructure evolution and reaction mechanism between the matrix and PT template was investigated systematically. The quench heat treatment experiment was designed and the microstructure was evaluated. The results showed that the plate-like PT template has relatively low thermal stability which would decompose to form Pb-rich liquid phase and Ti-rich region at the sintering temperature of 900 °C–1050 °C. Plate-like PT template reacted with the PZNNT matrix materials during the sintering process, which did not contribute to the grain growth orientation for PZNNT matrix. Finally, the mechanism of grain growth for the PZNNT ceramics with plate-like PT template is clarified. This work demonstrated that the thermal stability of plate-like template is one of the key factors for fabricating textured piezoelectric ceramics.

Original language	English
Pages (from-to)	470-478
Number of pages	9
Journal	Ceramics International
Volume	47
Issue number	1
DOIs	https://doi.org/10.1016/j.ceramint.2020.08.154
State	Published - 1 Jan 2021

Keywords

Microstructure evolution
PbTiO template
PZNNT matrix Materials
Texture ceramics

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@article{684bd25f67b0401f8b426241537dc274,

title = "Microstructure evolution and reaction mechanism of Pb(Zr1/2Ti1/2)O3-Pb(Zn1/3Nb2/3)O3–Pb(Ni1/3Nb2/3)O3 piezoelectric ceramics with plate-like PbTiO3 template",

abstract = "0.83 Pb(Zr1/2Ti1/2)O3-0.11Pb(Zn1/3Nb2/3)O3-0.06Pb(Ni1/3Nb2/3)O3 (PZNNT) samples with plate-like PbTiO3 (PT) template were prepared using tape casting technology. The microstructure evolution and reaction mechanism between the matrix and PT template was investigated systematically. The quench heat treatment experiment was designed and the microstructure was evaluated. The results showed that the plate-like PT template has relatively low thermal stability which would decompose to form Pb-rich liquid phase and Ti-rich region at the sintering temperature of 900 °C–1050 °C. Plate-like PT template reacted with the PZNNT matrix materials during the sintering process, which did not contribute to the grain growth orientation for PZNNT matrix. Finally, the mechanism of grain growth for the PZNNT ceramics with plate-like PT template is clarified. This work demonstrated that the thermal stability of plate-like template is one of the key factors for fabricating textured piezoelectric ceramics.",

keywords = "Microstructure evolution, PbTiO template, PZNNT matrix Materials, Texture ceramics",

author = "Leilei Li and Junting Liu and Shuyao Cao and Jie Xu and Changying Wu and Emilia Pawlikowska and Miko{\l}aj Szafran and Feng Gao",

note = "Publisher Copyright: {\textcopyright} 2020 Elsevier Ltd and Techna Group S.r.l.",

year = "2021",

month = jan,

day = "1",

doi = "10.1016/j.ceramint.2020.08.154",

language = "英语",

volume = "47",

pages = "470--478",

journal = "Ceramics International",

issn = "0272-8842",

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TY - JOUR

T1 - Microstructure evolution and reaction mechanism of Pb(Zr1/2Ti1/2)O3-Pb(Zn1/3Nb2/3)O3–Pb(Ni1/3Nb2/3)O3 piezoelectric ceramics with plate-like PbTiO3 template

AU - Li, Leilei

AU - Liu, Junting

AU - Cao, Shuyao

AU - Xu, Jie

AU - Wu, Changying

AU - Pawlikowska, Emilia

AU - Szafran, Mikołaj

AU - Gao, Feng

PY - 2021/1/1

Y1 - 2021/1/1

N2 - 0.83 Pb(Zr1/2Ti1/2)O3-0.11Pb(Zn1/3Nb2/3)O3-0.06Pb(Ni1/3Nb2/3)O3 (PZNNT) samples with plate-like PbTiO3 (PT) template were prepared using tape casting technology. The microstructure evolution and reaction mechanism between the matrix and PT template was investigated systematically. The quench heat treatment experiment was designed and the microstructure was evaluated. The results showed that the plate-like PT template has relatively low thermal stability which would decompose to form Pb-rich liquid phase and Ti-rich region at the sintering temperature of 900 °C–1050 °C. Plate-like PT template reacted with the PZNNT matrix materials during the sintering process, which did not contribute to the grain growth orientation for PZNNT matrix. Finally, the mechanism of grain growth for the PZNNT ceramics with plate-like PT template is clarified. This work demonstrated that the thermal stability of plate-like template is one of the key factors for fabricating textured piezoelectric ceramics.

AB - 0.83 Pb(Zr1/2Ti1/2)O3-0.11Pb(Zn1/3Nb2/3)O3-0.06Pb(Ni1/3Nb2/3)O3 (PZNNT) samples with plate-like PbTiO3 (PT) template were prepared using tape casting technology. The microstructure evolution and reaction mechanism between the matrix and PT template was investigated systematically. The quench heat treatment experiment was designed and the microstructure was evaluated. The results showed that the plate-like PT template has relatively low thermal stability which would decompose to form Pb-rich liquid phase and Ti-rich region at the sintering temperature of 900 °C–1050 °C. Plate-like PT template reacted with the PZNNT matrix materials during the sintering process, which did not contribute to the grain growth orientation for PZNNT matrix. Finally, the mechanism of grain growth for the PZNNT ceramics with plate-like PT template is clarified. This work demonstrated that the thermal stability of plate-like template is one of the key factors for fabricating textured piezoelectric ceramics.

KW - Microstructure evolution

KW - PbTiO template

KW - PZNNT matrix Materials

KW - Texture ceramics

UR - https://www.scopus.com/pages/publications/85090152164

U2 - 10.1016/j.ceramint.2020.08.154

DO - 10.1016/j.ceramint.2020.08.154

M3 - 文章

AN - SCOPUS:85090152164

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VL - 47

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Microstructure evolution and reaction mechanism of Pb(Zr_1/2Ti_1/2)O₃-Pb(Zn_1/3Nb_2/3)O₃–Pb(Ni_1/3Nb_2/3)O₃ piezoelectric ceramics with plate-like PbTiO₃ template

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