Mesoporous metal-organic frameworks with size-, shape-, and space-distribution-controlled pore structure

Weina Zhang; Yayuan Liu; Guang Lu; Yong Wang; Shaozhou Li; Chenlong Cui; Jin Wu; Zhiling Xu; Danbi Tian; Wei Huang; Joseph S. Ducheneu; W. David Wei; Hongyu Chen; Yanhui Yang; Fengwei Huo

doi:10.1002/adma.201405752

Mesoporous metal-organic frameworks with size-, shape-, and space-distribution-controlled pore structure

Weina Zhang
, Yayuan Liu
, Guang Lu
, Yong Wang
, Shaozhou Li
, Chenlong Cui
, Jin Wu
, Zhiling Xu
, Danbi Tian
, Wei Huang
, Joseph S. Ducheneu
, W. David Wei
, Hongyu Chen
, Yanhui Yang
, Fengwei Huo

Nanjing Tech University
Nanyang Technological University
University of Florida

Research output: Contribution to journal › Article › peer-review

246 Scopus citations

Abstract

Mesoporous Metal-organic frameworks (meso-MOFs) with size-, shape-, and space-distribution-controlled mesopores are obtained by a facile encapsulation and selective etching strategy of metal nanoparticles. Hierarchical or functionalized meso-MOFs are achieved by the above strategy. Interestingly, the functional meso-MOFs display higher catalytic activity originating from the mesopores existing in the MOFs, as well as good selectivity due to protection of the microporous frameworks.

Original language	English
Pages (from-to)	2923-2929
Number of pages	7
Journal	Advanced Materials
Volume	27
Issue number	18
DOIs	https://doi.org/10.1002/adma.201405752
State	Published - 13 May 2015
Externally published	Yes

Keywords

mesoporous materials
metal nanoparticles
metal-organic frameworks
molecular diffusion
selective catalysis

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10.1002/adma.201405752

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title = "Mesoporous metal-organic frameworks with size-, shape-, and space-distribution-controlled pore structure",

abstract = "Mesoporous Metal-organic frameworks (meso-MOFs) with size-, shape-, and space-distribution-controlled mesopores are obtained by a facile encapsulation and selective etching strategy of metal nanoparticles. Hierarchical or functionalized meso-MOFs are achieved by the above strategy. Interestingly, the functional meso-MOFs display higher catalytic activity originating from the mesopores existing in the MOFs, as well as good selectivity due to protection of the microporous frameworks.",

keywords = "mesoporous materials, metal nanoparticles, metal-organic frameworks, molecular diffusion, selective catalysis",

author = "Weina Zhang and Yayuan Liu and Guang Lu and Yong Wang and Shaozhou Li and Chenlong Cui and Jin Wu and Zhiling Xu and Danbi Tian and Wei Huang and Ducheneu, \{Joseph S.\} and Wei, \{W. David\} and Hongyu Chen and Yanhui Yang and Fengwei Huo",

note = "Publisher Copyright: {\textcopyright} 2015 WILEY-VCH Verlag GmbH \& Co. KGaA, Weinheim.",

year = "2015",

month = may,

day = "13",

doi = "10.1002/adma.201405752",

language = "英语",

volume = "27",

pages = "2923--2929",

journal = "Advanced Materials",

issn = "0935-9648",

publisher = "Wiley-Blackwell",

number = "18",

}

TY - JOUR

T1 - Mesoporous metal-organic frameworks with size-, shape-, and space-distribution-controlled pore structure

AU - Zhang, Weina

AU - Liu, Yayuan

AU - Lu, Guang

AU - Wang, Yong

AU - Li, Shaozhou

AU - Cui, Chenlong

AU - Wu, Jin

AU - Xu, Zhiling

AU - Tian, Danbi

AU - Huang, Wei

AU - Ducheneu, Joseph S.

AU - Wei, W. David

AU - Chen, Hongyu

AU - Yang, Yanhui

AU - Huo, Fengwei

PY - 2015/5/13

Y1 - 2015/5/13

N2 - Mesoporous Metal-organic frameworks (meso-MOFs) with size-, shape-, and space-distribution-controlled mesopores are obtained by a facile encapsulation and selective etching strategy of metal nanoparticles. Hierarchical or functionalized meso-MOFs are achieved by the above strategy. Interestingly, the functional meso-MOFs display higher catalytic activity originating from the mesopores existing in the MOFs, as well as good selectivity due to protection of the microporous frameworks.

AB - Mesoporous Metal-organic frameworks (meso-MOFs) with size-, shape-, and space-distribution-controlled mesopores are obtained by a facile encapsulation and selective etching strategy of metal nanoparticles. Hierarchical or functionalized meso-MOFs are achieved by the above strategy. Interestingly, the functional meso-MOFs display higher catalytic activity originating from the mesopores existing in the MOFs, as well as good selectivity due to protection of the microporous frameworks.

KW - mesoporous materials

KW - metal nanoparticles

KW - metal-organic frameworks

KW - molecular diffusion

KW - selective catalysis

UR - https://www.scopus.com/pages/publications/85027919818

U2 - 10.1002/adma.201405752

DO - 10.1002/adma.201405752

M3 - 文章

AN - SCOPUS:85027919818

SN - 0935-9648

VL - 27

SP - 2923

EP - 2929

JO - Advanced Materials

JF - Advanced Materials

IS - 18

ER -

Mesoporous metal-organic frameworks with size-, shape-, and space-distribution-controlled pore structure

Abstract

Keywords

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