Magnetic properties and evidence of a new spin-glass transition induced by Mn-doping in Tb2NiSi3

Xiao Jun Bai; Lu Yao Wang; Zhi Yan Pan; Rui Bo Song; Yao Cen Wang; Li Bing Duan; Xin Lin; Nikolai S. Perov; Chong De Cao

doi:10.1016/j.jmmm.2021.168396

Magnetic properties and evidence of a new spin-glass transition induced by Mn-doping in Tb₂NiSi₃

Xiao Jun Bai
, Lu Yao Wang
, Zhi Yan Pan
, Rui Bo Song
, Yao Cen Wang
, Li Bing Duan
, Xin Lin
, Nikolai S. Perov
, Chong De Cao

School of Materials Sience and Engineering

Northwestern Polytechnical University Xian
Polytechnical University
Lomonosov Moscow State University

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Abstract

It is extremely rare for the coexistence of two spin glass transitions in single phase materials. In the present paper, the structure and magnetic properties of Tb₂Ni_0.8Mn_0.2Si₃ were investigated. For comparison, the corresponding experimental results of Tb₂NiSi₃ compound were also provided. In the temperature dependence of dc susceptibility measurements, there are two anomaly transitions for both Tb₂Ni_0.8Mn_0.2Si₃ and Tb₂NiSi₃. Further studies on the frequency dependence of ac susceptibility show a new spin-glass transition at 14 K in Tb₂Ni_0.8Mn_0.2Si₃, except for the spin-glass transition at 8 K inheriting from Tb₂NiSi₃. This new spin-glass transition in Tb₂Ni_0.8Mn_0.2Si₃ is absent in Tb₂NiSi₃. It takes place below the long-range magnetic ordered phase transition and shows cluster spin glass behaviors, and it is attributed to the introduction of Mn ions into the intermetallic compound.

Original language	English
Article number	168396
Journal	Journal of Magnetism and Magnetic Materials
Volume	539
DOIs	https://doi.org/10.1016/j.jmmm.2021.168396
State	Published - 1 Dec 2021

Keywords

Magnetic properties
Phase transition
Spin glass
TbNiMnSi

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10.1016/j.jmmm.2021.168396

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@article{e020391d1b204179b6c658d267c82933,

title = "Magnetic properties and evidence of a new spin-glass transition induced by Mn-doping in Tb2NiSi3",

abstract = "It is extremely rare for the coexistence of two spin glass transitions in single phase materials. In the present paper, the structure and magnetic properties of Tb2Ni0.8Mn0.2Si3 were investigated. For comparison, the corresponding experimental results of Tb2NiSi3 compound were also provided. In the temperature dependence of dc susceptibility measurements, there are two anomaly transitions for both Tb2Ni0.8Mn0.2Si3 and Tb2NiSi3. Further studies on the frequency dependence of ac susceptibility show a new spin-glass transition at 14 K in Tb2Ni0.8Mn0.2Si3, except for the spin-glass transition at 8 K inheriting from Tb2NiSi3. This new spin-glass transition in Tb2Ni0.8Mn0.2Si3 is absent in Tb2NiSi3. It takes place below the long-range magnetic ordered phase transition and shows cluster spin glass behaviors, and it is attributed to the introduction of Mn ions into the intermetallic compound.",

keywords = "Magnetic properties, Phase transition, Spin glass, TbNiMnSi",

author = "Bai, \{Xiao Jun\} and Wang, \{Lu Yao\} and Pan, \{Zhi Yan\} and Song, \{Rui Bo\} and Wang, \{Yao Cen\} and Duan, \{Li Bing\} and Xin Lin and Perov, \{Nikolai S.\} and Cao, \{Chong De\}",

note = "Publisher Copyright: {\textcopyright} 2021 Elsevier B.V.",

year = "2021",

month = dec,

day = "1",

doi = "10.1016/j.jmmm.2021.168396",

language = "英语",

volume = "539",

journal = "Journal of Magnetism and Magnetic Materials",

issn = "0304-8853",

publisher = "Elsevier B.V.",

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TY - JOUR

T1 - Magnetic properties and evidence of a new spin-glass transition induced by Mn-doping in Tb2NiSi3

AU - Bai, Xiao Jun

AU - Wang, Lu Yao

AU - Pan, Zhi Yan

AU - Song, Rui Bo

AU - Wang, Yao Cen

AU - Duan, Li Bing

AU - Lin, Xin

AU - Perov, Nikolai S.

AU - Cao, Chong De

PY - 2021/12/1

Y1 - 2021/12/1

N2 - It is extremely rare for the coexistence of two spin glass transitions in single phase materials. In the present paper, the structure and magnetic properties of Tb2Ni0.8Mn0.2Si3 were investigated. For comparison, the corresponding experimental results of Tb2NiSi3 compound were also provided. In the temperature dependence of dc susceptibility measurements, there are two anomaly transitions for both Tb2Ni0.8Mn0.2Si3 and Tb2NiSi3. Further studies on the frequency dependence of ac susceptibility show a new spin-glass transition at 14 K in Tb2Ni0.8Mn0.2Si3, except for the spin-glass transition at 8 K inheriting from Tb2NiSi3. This new spin-glass transition in Tb2Ni0.8Mn0.2Si3 is absent in Tb2NiSi3. It takes place below the long-range magnetic ordered phase transition and shows cluster spin glass behaviors, and it is attributed to the introduction of Mn ions into the intermetallic compound.

AB - It is extremely rare for the coexistence of two spin glass transitions in single phase materials. In the present paper, the structure and magnetic properties of Tb2Ni0.8Mn0.2Si3 were investigated. For comparison, the corresponding experimental results of Tb2NiSi3 compound were also provided. In the temperature dependence of dc susceptibility measurements, there are two anomaly transitions for both Tb2Ni0.8Mn0.2Si3 and Tb2NiSi3. Further studies on the frequency dependence of ac susceptibility show a new spin-glass transition at 14 K in Tb2Ni0.8Mn0.2Si3, except for the spin-glass transition at 8 K inheriting from Tb2NiSi3. This new spin-glass transition in Tb2Ni0.8Mn0.2Si3 is absent in Tb2NiSi3. It takes place below the long-range magnetic ordered phase transition and shows cluster spin glass behaviors, and it is attributed to the introduction of Mn ions into the intermetallic compound.

KW - Magnetic properties

KW - Phase transition

KW - Spin glass

KW - TbNiMnSi

UR - https://www.scopus.com/pages/publications/85113285683

U2 - 10.1016/j.jmmm.2021.168396

DO - 10.1016/j.jmmm.2021.168396

M3 - 文章

AN - SCOPUS:85113285683

SN - 0304-8853

VL - 539

JO - Journal of Magnetism and Magnetic Materials

JF - Journal of Magnetism and Magnetic Materials

M1 - 168396

ER -

Magnetic properties and evidence of a new spin-glass transition induced by Mn-doping in Tb₂NiSi₃

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Keywords

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