Hafnium Sulfide Nanosheets for Ultrafast Photonic Device

Jinde Yin, Fangxiang Zhu, Jintao Lai, Hao Chen, Mengyu Zhang, Jiaqiang Zhang, Jintao Wang, Tingchao He, Bo Zhang, Jianping Yuan, Peiguang Yan, Shuangchen Ruan

Research output: Contribution to journalArticlepeer-review

67 Scopus citations

Abstract

Group IVB transition metal dichalcogenides (TMDs) have attracted significant interests in photoelectronics due to their predictable superior physical properties compared to group VIB (Mo and W) TMDs. However, the nonlinear optical properties and ultrafast photonic devices based on group IVB TMDs remained unexplored so far. Herein, the nonlinear optical absorption of HfS 2 nanosheets (NSs) prepared by liquid exfoliation is demonstrated. The usage of HfS 2 as a new ultrafast photonic device for high-energy and ultrashort pulse generation in a fiber laser is reported for the first time. A photonic crystal fiber (PCF) assisted deposition method is presented for the fabrication of an HfS 2 -microfiber integrated saturable absorber (SA) device with precisely controllable light–matter interaction, which can benefit the output of the device. The HfS 2 -microfiber SA device shows modulation depth of 15.7% and exhibits outstanding ultrashort pulse generation performance with pulse duration of 221.7 fs in the communication band. The experimental results suggest that HfS 2 presents highly nonlinear optical absorption and can be developed into an excellent candidate of SA devices for the development of HfS 2 -based ultrafast photonics.

Original languageEnglish
Article number1801303
JournalAdvanced Optical Materials
Volume7
Issue number5
DOIs
StatePublished - 5 Mar 2019
Externally publishedYes

Keywords

  • hafnium sulfide
  • nonlinear optics
  • ultrafast photonics

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