Corrosion behavior of bulk (Zr                         58                         Nb                         3                         Cu                         16                         Ni                         13                         Al                         10                         )                         100-x                         Y                         x                          (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid

Liusi Yu; Junlei Tang; Hu Wang; Yingying Wang; Jichao Qiao; Mihai Apreutesei; Bernard Normand

doi:10.1016/j.corsci.2019.01.016

Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid

Liusi Yu
, Junlei Tang
, Hu Wang
, Yingying Wang
, Jichao Qiao
, Mihai Apreutesei
, Bernard Normand

School of Mechanics,Civil Engineering and Architecture

Research output: Contribution to journal › Article › peer-review

55 Scopus citations

Abstract

Bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses exhibited good passivation ability and outstanding corrosion resistance in de-aerated 0.5 mol/L H ₂ SO ₄ solution. It was mainly beneficial from the stable passive film which mainly consisted of ZrO ₂ and Al ₂ O ₃ . However, the defects concentration in the passive films increased with the increasing yttrium content in the Zr-based BMGs. The yttrium additions improved the electrochemical homogeneities of the Zr-based BMGs, but facilitated the dissolution of Cu, resulting in a slight deterioration of corrosion resistance of the Zr-based BMGs.

Original language	English
Pages (from-to)	42-53
Number of pages	12
Journal	Corrosion Science
Volume	150
DOIs	https://doi.org/10.1016/j.corsci.2019.01.016
State	Published - 15 Apr 2019

Keywords

Localized electrochemical impedance spectroscopy
Mott-Schottky
Scanning vibrating electrode technique
X-ray photoelectron spectroscopy
Yttrium
Zr-based bulk metallic glasses

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10.1016/j.corsci.2019.01.016

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Yu, L., Tang, J., Wang, H., Wang, Y., Qiao, J., Apreutesei, M., & Normand, B. (2019). Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid Corrosion Science, 150, 42-53. https://doi.org/10.1016/j.corsci.2019.01.016

Yu, Liusi ; Tang, Junlei ; Wang, Hu et al. / Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid In: Corrosion Science. 2019 ; Vol. 150. pp. 42-53.

@article{bfccb4425e80436192fd17e8c45f19d4,

title = " Corrosion behavior of bulk (Zr 58 Nb 3 Cu 16 Ni 13 Al 10 ) 100-x Y x (x = 0, 0.5, 2.5 at.\%) metallic glasses in sulfuric acid ",

abstract = " Bulk (Zr 58 Nb 3 Cu 16 Ni 13 Al 10 ) 100-x Y x (x = 0, 0.5, 2.5 at.\%) metallic glasses exhibited good passivation ability and outstanding corrosion resistance in de-aerated 0.5 mol/L H 2 SO 4 solution. It was mainly beneficial from the stable passive film which mainly consisted of ZrO 2 and Al 2 O 3 . However, the defects concentration in the passive films increased with the increasing yttrium content in the Zr-based BMGs. The yttrium additions improved the electrochemical homogeneities of the Zr-based BMGs, but facilitated the dissolution of Cu, resulting in a slight deterioration of corrosion resistance of the Zr-based BMGs.",

keywords = "Localized electrochemical impedance spectroscopy, Mott-Schottky, Scanning vibrating electrode technique, X-ray photoelectron spectroscopy, Yttrium, Zr-based bulk metallic glasses",

author = "Liusi Yu and Junlei Tang and Hu Wang and Yingying Wang and Jichao Qiao and Mihai Apreutesei and Bernard Normand",

note = "Publisher Copyright: {\textcopyright} 2019 Elsevier Ltd",

year = "2019",

month = apr,

day = "15",

doi = "10.1016/j.corsci.2019.01.016",

language = "英语",

volume = "150",

pages = "42--53",

journal = "Corrosion Science",

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Yu, L, Tang, J, Wang, H, Wang, Y, Qiao, J, Apreutesei, M & Normand, B 2019, ' Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid ', Corrosion Science, vol. 150, pp. 42-53. https://doi.org/10.1016/j.corsci.2019.01.016

Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid . / Yu, Liusi; Tang, Junlei; Wang, Hu et al.
In: Corrosion Science, Vol. 150, 15.04.2019, p. 42-53.

Research output: Contribution to journal › Article › peer-review

TY - JOUR

T1 - Corrosion behavior of bulk (Zr 58 Nb 3 Cu 16 Ni 13 Al 10 ) 100-x Y x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid

AU - Yu, Liusi

AU - Tang, Junlei

AU - Wang, Hu

AU - Wang, Yingying

AU - Qiao, Jichao

AU - Apreutesei, Mihai

AU - Normand, Bernard

PY - 2019/4/15

Y1 - 2019/4/15

N2 - Bulk (Zr 58 Nb 3 Cu 16 Ni 13 Al 10 ) 100-x Y x (x = 0, 0.5, 2.5 at.%) metallic glasses exhibited good passivation ability and outstanding corrosion resistance in de-aerated 0.5 mol/L H 2 SO 4 solution. It was mainly beneficial from the stable passive film which mainly consisted of ZrO 2 and Al 2 O 3 . However, the defects concentration in the passive films increased with the increasing yttrium content in the Zr-based BMGs. The yttrium additions improved the electrochemical homogeneities of the Zr-based BMGs, but facilitated the dissolution of Cu, resulting in a slight deterioration of corrosion resistance of the Zr-based BMGs.

AB - Bulk (Zr 58 Nb 3 Cu 16 Ni 13 Al 10 ) 100-x Y x (x = 0, 0.5, 2.5 at.%) metallic glasses exhibited good passivation ability and outstanding corrosion resistance in de-aerated 0.5 mol/L H 2 SO 4 solution. It was mainly beneficial from the stable passive film which mainly consisted of ZrO 2 and Al 2 O 3 . However, the defects concentration in the passive films increased with the increasing yttrium content in the Zr-based BMGs. The yttrium additions improved the electrochemical homogeneities of the Zr-based BMGs, but facilitated the dissolution of Cu, resulting in a slight deterioration of corrosion resistance of the Zr-based BMGs.

KW - Localized electrochemical impedance spectroscopy

KW - Mott-Schottky

KW - Scanning vibrating electrode technique

KW - X-ray photoelectron spectroscopy

KW - Yttrium

KW - Zr-based bulk metallic glasses

UR - https://www.scopus.com/pages/publications/85060326951

U2 - 10.1016/j.corsci.2019.01.016

DO - 10.1016/j.corsci.2019.01.016

M3 - 文章

AN - SCOPUS:85060326951

SN - 0010-938X

VL - 150

SP - 42

EP - 53

JO - Corrosion Science

JF - Corrosion Science

ER -

Yu L, Tang J, Wang H, Wang Y, Qiao J, Apreutesei M et al. Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid Corrosion Science. 2019 Apr 15;150:42-53. doi: 10.1016/j.corsci.2019.01.016

Corrosion behavior of bulk (Zr ₅₈ Nb ₃ Cu ₁₆ Ni ₁₃ Al ₁₀ ) _100-x Y _x (x = 0, 0.5, 2.5 at.%) metallic glasses in sulfuric acid

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