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A novel dielectric barrier discharge reactor with photocatalytic electrode based on sintered metal fibers for abatement of xylene

  • Zhiping Ye
  • , Chunxia Wang
  • , Zhenhua Shao
  • , Qing Ye
  • , Yi He
  • , Yao Shi
  • Key Laboratory of Biomass Chemical Engineering

Research output: Contribution to journalArticlepeer-review

28 Scopus citations

Abstract

A novel dielectric barrier discharge (DBD) reactor was made for the abatement of xylene. This reactor has a photocatalytic electrode prepared by a modified anodic oxidation method which was proposed in this work. The photocatalytic electrode has nano-TiO2 deposited on sintered metal fiber (SMF). The reactor using the nano-TiO2/SMF electrode shows much better performance in abating xylene compared with reactors using other electrodes such as resistance wire or SMF. The conversion ratio of xylene reaches 92.7% in the novel reactor at a relatively voltage (23.6kV). This ratio is much higher than the conversion ratios of xylene in the traditional reactors with resistance wire or SMF electrodes, which are ∼64.7%. The selectivity of CO2 of the reactor using the nano-TiO2/SMF electrode (300pps, 23.6kV) was observed to be 86.6%, which is about twice as large as that of a traditional reactor using a resistance wire electrode. If a traditional DBD reactor is replaced by the novel reactor, at the same specific input energy, the energy yield can increase from 0.391 to 0.556mg/kJ. Finally, the xylene decomposition mechanism with the nano-TiO2/SMF electrode was also briefly discussed.

Original languageEnglish
Pages (from-to)216-223
Number of pages8
JournalJournal of Hazardous Materials
Volume241-242
DOIs
StatePublished - 30 Nov 2012
Externally publishedYes

Keywords

  • Anodic oxidation
  • Dielectric barrier discharge
  • Nano-TiO/SMF electrode
  • Ti
  • Xylene

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