Abstract
A novel dielectric barrier discharge (DBD) reactor was made for the abatement of xylene. This reactor has a photocatalytic electrode prepared by a modified anodic oxidation method which was proposed in this work. The photocatalytic electrode has nano-TiO2 deposited on sintered metal fiber (SMF). The reactor using the nano-TiO2/SMF electrode shows much better performance in abating xylene compared with reactors using other electrodes such as resistance wire or SMF. The conversion ratio of xylene reaches 92.7% in the novel reactor at a relatively voltage (23.6kV). This ratio is much higher than the conversion ratios of xylene in the traditional reactors with resistance wire or SMF electrodes, which are ∼64.7%. The selectivity of CO2 of the reactor using the nano-TiO2/SMF electrode (300pps, 23.6kV) was observed to be 86.6%, which is about twice as large as that of a traditional reactor using a resistance wire electrode. If a traditional DBD reactor is replaced by the novel reactor, at the same specific input energy, the energy yield can increase from 0.391 to 0.556mg/kJ. Finally, the xylene decomposition mechanism with the nano-TiO2/SMF electrode was also briefly discussed.
| Original language | English |
|---|---|
| Pages (from-to) | 216-223 |
| Number of pages | 8 |
| Journal | Journal of Hazardous Materials |
| Volume | 241-242 |
| DOIs | |
| State | Published - 30 Nov 2012 |
| Externally published | Yes |
Keywords
- Anodic oxidation
- Dielectric barrier discharge
- Nano-TiO/SMF electrode
- Ti
- Xylene
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